The AutoCompleteMode in Windows Forms does not (as of now) support filtering with regular expression or matching from the middle. It supports prefix filtering only.
The API to reset the autocomplete options as you type is IAutoCompleteDropDown::ResetEnumerator. You need to call it in the TextChanged event.
On Windows Vista or later you can call IAutoComplete2::SetOptions with ACO_NOPREFIXFILTERING to disable prefix filtering.
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