If it's not a typed dataset, then you probably want to do something like this, using the Linq-to-DataSet extension methods:
var distinctValues = dsValues.AsEnumerable()
.Select(row => new {
attribute1_name = row.Field<string>("attribute1_name"),
attribute2_name = row.Field<string>("attribute2_name")
})
.Distinct();
Make sure you have a using System.Data;
statement at the beginning of your code in order to enable the Linq-to-Dataset extension methods.
Hope this helps!
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