Here's a great article that should help you build your algorithm
http://www.codeproject.com/KB/datetime/christianholidays.aspx
Based on this example, you should be able to write:
DateTime goodFriday = EasterSunday(DateTime.Now.Year).AddDays(-2);
Full Example:
public static DateTime EasterSunday(int year)
{
int day = 0;
int month = 0;
int g = year % 19;
int c = year / 100;
int h = (c - (int)(c / 4) - (int)((8 * c + 13) / 25) + 19 * g + 15) % 30;
int i = h - (int)(h / 28) * (1 - (int)(h / 28) * (int)(29 / (h + 1)) * (int)((21 - g) / 11));
day = i - ((year + (int)(year / 4) + i + 2 - c + (int)(c / 4)) % 7) + 28;
month = 3;
if (day > 31)
{
month++;
day -= 31;
}
return new DateTime(year, month, day);
}
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